A Test of the Utility of Plane Waves for the Study of Molecules from First Principles

نویسندگان

  • Andrew M. Rappe
  • J. D. Joannopoulos
  • P. A. Bash
چکیده

This paper studies the applicability of a plane-wave basis set for density functional calculations of the properties of molecules from first principles. The main features of the plane-wave method are described, including pseudopotentials and supercells. The results for a number of small molecules are reported. The close agreement with experiment and with a standard method of quantum chemistry calculation indicates the promise which this method holds for chemical and biochemical first-principles computations.

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تاریخ انتشار 2001